Water dynamics in C–S–H and M-S-H cement pastes: A revised jump-diffusion and rotation-diffusion model

نویسندگان

چکیده

The Quasi-Elastic Neutron Scattering (QENS) spectra from four cement pastes are re-analyzed by a new revised jump-diffusion and rotation-diffusion model (rJRM). From the QENS fit, it can be seen that rJRM is an improved to fit within whole detected neutron energy transfer scattering vector. By fitting, structure parameters extracted show both additives aluminum-silicate nanotubes (ASN) carboxyl group functionalized ASN (ASN-COOH) improve magnesium-silicate-hydrate (M-S-H) toward calcium-silicate-hydrate (C–S–H) direction in mechanical properties, but improvement weakened with decreasing temperatures. dynamical there dynamic anomaly near 230 K not only translational also rotational diffusion of water confined all investigated samples. compared those results obtained using other models. • (rJRM) collected on at temperatures 210 - 280 E between -120 120 μeV Q 0.3 1.9 Å-1. ASN-COOH M-S-H C-S-H fitted anomalies for water.

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

The Voter Model and Jump Diffusion

Opinions, and subsequently opinion dynamics, depend not just on interactions among individuals, but also on external influences such as the mass media. The dependence on local interactions, however, has received considerably more attention. In this paper, we use the classical voter model as a basis, and extend it to include external influences. We show that this new model can be understood usin...

متن کامل

Closed formulas for the price and sensitivities of European options under a double exponential jump diffusion model

We derive closed formulas for the prices of European options andtheir sensitivities when the underlying asset follows a double-exponentialjump diffusion model, as considered by S. Kou in 2002. This author hasderived the option price by making use of double series where each termrequires the computation of a sequence of special functions, such thatthe implementation remains difficult for a large...

متن کامل

A Jump-Diffusion Model for Option Pricing

Brownian motion and normal distribution have been widely used in the Black–Scholes option-pricing framework to model the return of assets. However, two puzzles emerge from many empirical investigations: the leptokurtic feature that the return distribution of assets may have a higher peak and two (asymmetric) heavier tails than those of the normal distribution, and an empirical phenomenon called...

متن کامل

A Nuclear Magnetic Resonance Pulsed Field Gradient Study of Self-Diffusion of Water in Hydrated Cement Pastes

The results of oneand two-dimensional H nuclear magnetic resonance (NMR) pulsed field gradient (PFG) diffusometry studies of water in white cement paste with a water-tocement ratio 0.4 and aged from 1 day to 1 year are reported. The study shows that the NMRPFG method is primarily sensitive to the capillary porosity. Data is fit on the basis of a lognormal pore size distribution with pore size d...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Physica B-condensed Matter

سال: 2022

ISSN: ['1873-2135', '0921-4526']

DOI: https://doi.org/10.1016/j.physb.2021.413542